The relationship between recombination, chemical activation and unimolecular dissociation rate coefficients
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چکیده
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15 صفحه اولPressure effects on bimolecular recombination and unimolecular dissociation reactions
The treatment of pressure effects on bimolecular recombinations and unimolecular dissociations is discussed. The analysis of recombination and dissociation reactions is made by showing how the nonequilibrium energy ~E! and angular momentum ~J!-dependent steady-state population distribution functions for the two reactions are related to each other and to the equilibrium population distribution f...
متن کاملThe dissociation/recombination reaction CH4 (+M) ⇔ CH3 + H (+M): a case study for unimolecular rate theory.
The dissociation/recombination reaction CH(4) (+M) ⇔ CH(3) + H (+M) is modeled by statistical unimolecular rate theory completely based on dynamical information using ab initio potentials. The results are compared with experimental data. Minor discrepancies are removed by fine-tuning theoretical energy transfer data. The treatment accounts for transitional mode dynamics, adequate centrifugal ba...
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ژورنال
عنوان ژورنال: The Journal of Chemical Physics
سال: 1989
ISSN: 0021-9606,1089-7690
DOI: 10.1063/1.455783